Triphosgene

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Triphosgene
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Template:Longitem C3Cl6O3
Molar mass 296.748 g/mol
Appearance white solid
Density 1.780 g/cm3
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Solubility *soluble in dichloromethane[1]
  • soluble in THF[2]
  • soluble in toluene[3]

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Triphosgene (bis(trichloromethyl) carbonate (BTC)) is a chemical compound with the formula OC(OCCl3)2. It is used as a solid substitute for phosgene, which is a gas and diphosgene, which is a liquid.[5][6] Triphosgene is stable up to 200 °C.[7] Triphosgene is used in a variety of halogenation reactions.[8]

Preparation

This compound is commercially available. It is prepared by exhaustive free radical chlorination of dimethyl carbonate:[6]

CH3OCO2CH3 + 6 Cl2 → CCl3OCO2CCl3 + 6 HCl

Triphosgene can be easily recrystallized from hot hexanes.

Uses

Triphosgene is used as a reagent in organic synthesis as a source of CO2+. It behaves like phosgene, to which it cracks thermally:

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Alcohols are converted to carbonates. Primary and secondary amines are converted to ureas and isocyanates.[6][7][9][10]

Triphosgene has been used to synthesize chlorides.[8] Some Alkyl chlorides are prepared by treating alcohols with a mixture of triphosgene and pyridine. Alkyl dichlorides and trichlorides can similarly be synthesized using triphosgene. Vinyl chlorides are synthesized from ketones using triphosgene and DMF to form a Vilsmeier reagent, followed by a ring opening by chloride ions. Aryl chlorides can also be produced using a Vilsmeier reagent from triphosgene and DMF.

Safety

The vapor pressure of Triphosgene is sufficiently high for it to reach concentrations that are considered toxicologically unsafe.[11] While several properties of triphosgene are not yet readily available, it is known that it is very toxic if inhaled. A toxic gas is emitted if it comes in contact with water.[12] There is a lack of information and variability regarding the proper handling of triphosgene. It is assumed to have the same risks as phosgene.[13][14]

See also

References

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  4. a b c Sigma-Aldrich Co., Triphosgene.
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External links